去除有机质对城市浅水湖泊氮磷释放特征的影响
作者:
中图分类号:

X171

基金项目:

国家自然科学基金项目“微流体污染物氨硝燃料电池层流界面膜功能特性研究”(51768019)


Effects of Organic Matter Removal on Nitrogen and Phosphorus Release Characteristics from Surface Sediments in Urban Shallow Lakes
Author:
  • 摘要
  • | |
  • 访问统计
  • |
  • 参考文献 [31]
  • |
  • 相似文献 [20]
  • | | |
  • 文章评论
    摘要:

    [目的] 分析南昌市浅水湖泊象湖表层沉积物的释放特征及有机质对氮、磷释放的影响,为城市内浅水湖泊治理中富营养化控制提供理论依据。[方法] 通过释放动力学试验以及释放潜能试验研究了城市浅水湖泊氨氮(NH4+-N)和溶解性活性磷(SRP)的释放特征,以及与通过H2O2去除有机质后的释放特征进行了对比。[结果] 去除前后的氮磷的释放速率都是先由一个较快的过程逐渐变慢最后趋于稳定达到最大释放量(Qmax)。去除有机质后NH4+-N的释放平衡时间缩短,SRP则几乎不变。去除有机质后,NH4+-N的最大释放量(Qmax)与有机质含量呈显著正相关,而SRP与有机质无显著相关性。[结论] 影响沉积物氮磷释放的因素多样,其中高等水生植物丰富的区域对磷的释放有明显的抑制作用。沉积物有机质的含量越高沉积物氮的最大释放量(Qmax)也越高,磷的的最大释放量(Qmax)则受有机质含量、活性、组成成分、吸附与结合的铁铝磷含量等因素共同影响。

    Abstract:

    [Objective] The release characteristics of surface sediments in shallow lakes of a city and the influence of organic matter on nitrogen and phosphorus release were analyzed to provide a theoretical basis for eutrophication control of shallow lakes.[Methods] The release characteristics of ammonia nitrogen (NH4+-N) and soluble reactive phosphorus (SRP) were studied in a shallow lake through a release kinetics experiment and a release potential experiment. Results were compared with the release characteristics after organic matter was removed by H2O2.[Results] The release rate of nitrogen and phosphorus before and after the removal of organic matter initially slowed down from a faster process, and finally stabilized to reach the maximum release rate. After the removal of organic matter, the release equilibrium time of NH4+-N was shortened, while SRP was almost unchanged. After removing organic matter, the maximum release of NH4+-N was significantly positively correlated with the organic matter content, while SRP had no significant correlation with organic matter.[Conclusion] Various factors influence the release of nitrogen and phosphorus in sediments. Areas rich in higher aquatic plants have a significant inhibitory effect on the release of phosphorus. The higher the content of organic matter in sediments, the higher the maximum release of nitrogen from sediments. The maximum release of phosphorus is affected by factors such as organic matter content, activity, composition, and adsorption, and the combined effects of iron, aluminum, and phosphorus content.

    参考文献
    [1] 雷沛, 张洪, 王超, 等.沉积物-水界面污染物迁移扩散的研究进展[J].湖泊科学, 2018, 30(6):1489-1508.
    [2] 陈洁, 许海, 詹旭, 等.湖泊沉积物-水界面磷的迁移转化机制与定量研究方法[J].湖泊科学, 2019(4):907-918.
    [3] 曹琳, 吉芳英, 林茂, 等.有机质对三峡库区消落区沉积物磷释放的影响[J].环境科学研究, 2011, 24(2):185-190.
    [4] 文林, 陈滢, 刘敏.氮氧化物气体的产生及其对厌氧氨氧化的影响研究[J].环境科学与技术, 2012, 35(4):99-103.
    [5] 胡玲珍, 陈振楼.河口沉积物反硝化反应影响因子综述[J].环境科学动态, 2003, 28(4):41-43.
    [6] 吴金浩, 刘桂英, 王年斌, 等.辽东湾北部海域表层沉积物氧化还原电位及其主要影响因素[J].沉积学报, 2012, 30(2):333-339.
    [7] 陈春丽, 戴星照, 曾桐辉, 等.城市内湖表层沉积物中有机氯农药残留特征及风险评价:以鄱阳湖生态经济区南昌市象湖为例[J].长江流域资源与环境, 2015, 24(12):2076-2084.
    [8] 李文华, 刘小真, 熊戬, 等.南昌市象湖水质监测[J].环境与健康杂志, 2013, 30(11):987.
    [9] 刘鹄, 孟婷, 程文, 等.汤浦水库沉积物碳、氮、磷的分布与评价[J].水土保持通报, 2017, 37(2):333-338.
    [10] Ruban V, López-Sánchez J F, Pardo P, et al. Harmonized protocol and certified reference material for the determination of extractable contents of phosphorus in freshwater sediments:A synthesis of recent works[J]. Fresenius' Journal of Analytical Chemistry, 2001, 370(2/3):224-228.
    [11] 李法松, 韩铖, 林大松, 等.安庆沿江湖泊及长江安庆段沉积物重金属污染特征及生态风险评价[J].农业环境科学学报, 2017, 36(3):574-582.
    [12] 宋鑫莱, 王耀晶, 张琢, 等.有机质的去除对磷酸盐稳定土壤铅的影响[J].农业环境科学学报, 2015, 34(8):1522-1527.
    [13] 易文利.湖泊沉积物中有机质含量对释放磷的影响[J].科学技术与工程, 2011, 11(26):6401-6404.
    [14] 王圣瑞, 赵海超, 王娟, 等.有机质对湖泊沉积物不同形态氮释放动力学影响研究[J].环境科学学报, 2012, 32(2):332-340.
    [15] Morin J, Morse J W. Ammonium release from resuspended sediments in the Laguna Madre estuary[J]. Marine Chemistry, 1999, 65(1/2):97-110.
    [16] 国家环境保护总局《水和废水监测分析方法》编委会.水和废水监测分析方法[M].4版, 北京:中国环境科学出版社, 2002:279-281.
    [17] 易文利, 王圣瑞, 金相灿, 等.去除轻组有机质对湖泊沉积物磷释放速率的影响研究[J].南开大学学报(自然科学版):2008, 41(4):1-7.
    [18] Aminot A, Andrieux F. Concept and determination of exchangeable phosphate in aquatic sediments[J]. Water Research, 1996, 30(11):2805-2811.
    [19] 黄威, 刘星, 赵丽, 等.岱海沉积物内源磷释放特征的研究[J].环境科学研究, 2020, 33(9):2094-2102.
    [20] 苏青青, 宋林旭, 刘德富, 等.三峡水库香溪河沉积物氮含量和氨氮释放特征[J].水生态学杂志, 2019, 40(3):1-7.
    [21] Cyr H, McCabe S K, Nürnberg G K. Phosphorus sorption experiments and the potential for internal phosphorus loading in littoral areas of a stratified lake[J].Water Research, 2009, 43(6):1654-1666.
    [22] Blair G, Lefroy R, Lisle L. Soil carbon fractions based on their degree of oxidation, and the development of a carbon management index for agricultural systems[J]. Australian Journal of Agricultural Research, 1995, 46(7):393-406.
    [23] 梁重山, 杨党志, 刘丛强, 等.土壤有机质对菲的吸附-解吸平衡的影响[J].高等学校化学学报, 2005, 26(4):671-676.
    [24] 屠晓翠, 蔡妙珍, 孙建国.大型水生植物对污染水体的净化作用和机理[J].安徽农业科学, 2006, 34(12):2843-2844.
    [25] 杨诗卡.水生植物根系有机酸驱动沉积物氮、磷转化机制[D].陕西西安:西安工业大学, 2019:24-28.
    [26] 汤志凯, 张毅敏, 杨飞, 等.3种水生植物腐解过程中磷营养物质迁移、转化过程研究[J].环境科学学报, 2019, 39(3):716-721.
    [27] 金丹越, 王圣瑞, 步青云.长江中下游浅水湖泊沉积物磷释放动力学[J].生态环境, 2007, 16(3):725-729.
    [28] 彭杰, 张杨珠, 周清, 等.去除有机质对土壤光谱特性的影响[J].土壤, 2006, 38(4):453-458.
    [29] 张桃林, 高超, 吴蔚东.氧化还原条件对土壤磷素固定与释放的影响[J].土壤学报, 2002, 39(4):542-549.
    [30] Slomp C P, Malschaert J F P, Van Raaphorst W. The role of adsorption in sediment-water exchange of phosphate in North Sea continental margin sediments[J]. Limnology and Oceanography, 1998, 43(5):832-846.
    [31] 赵海超, 王圣瑞, 张莉, 等.有机质含量及其组分对洱海沉积物磷吸附-释放影响[J].环境科学学报, 2014, 34(9):2346-2354.
    引证文献
    网友评论
    网友评论
    分享到微博
    发 布
引用本文

向速林,吴涛哲,龚聪远,吴代赦.去除有机质对城市浅水湖泊氮磷释放特征的影响[J].水土保持通报,2021,41(5):9-14,74

复制
分享
文章指标
  • 点击次数:461
  • 下载次数: 1047
  • HTML阅读次数: 0
  • 引用次数: 0
历史
  • 收稿日期:2021-03-18
  • 最后修改日期:2021-06-01
  • 在线发布日期: 2021-10-25